Laser-driven feedback effects reveal new ways to engineer conductivity in strongly interacting systems

Atomic illustration with electrons (Courtesy: Shutterstock/Agsandrew)

According to band theory, materials with partially filled energy bands and unpaired electrons should conduct electricity, but in Mott insulators this rule is broken. In these materials, the repulsion between electrons is so strong that they cannot move freely and become localized. When sufficient energy is supplied (for example by light), electrons can form a doublon (two electrons on one site) and a hole (an empty site). These excitations can move, enabling electrical conductivity.

A key question for Mott insulators is how these charge carriers are created and what controls their production. Traditionally, two regimes were known: multiphoton absorption, where several photons combine their energy, and tunnelling, where a strong electric field drives electrons across the gap.

In this work, the authors show that there are actually four regimes: multiphoton, tunnelling, a cooperative regime where the two processes work together, and an incoherent regime where weak fields and scattering dominate. They also show that the energy gap (the cost to create a doubloon-hole pair) is not fixed, but changes during the process because the generated carriers modify the system. This creates a feedback loop, making the dynamics nonlinear and time-dependent. As a result, carrier production can either slow down or suddenly speed up, even making the system more efficient without changing the driving field.

The behaviour depends on field strength, frequency, dissipation, and time, and each mechanism can be identified by its distinct momentum pattern. By tuning laser parameters, the system’s properties can be controlled in real time. Overall, this work shows that light can be used to dynamically reshape and control strongly interacting materials, opening possibilities for ultrafast, light-driven technologies.

Do you want to learn more about this topic?

PLP-Logo-2.png, find out more. Quantum frustration in organic Mott insulators: from spin liquids to unconventional superconductors by B J Powell and Ross H McKenzie (2011)